جهت دسترسی به کاربرگه ی زیر، از این لینک استفاده کنید. http://dl.pgu.ac.ir/handle/Hannan/81872
Title: Nanocrystals of cesium lead halide perovskites (CsPbX3, X = Cl, Br, and I): novel optoelectronic materials showing bright emission with wide color gamut
Keywords: Science & Technology;Physical Sciences;Technology;Chemistry, Multidisciplinary;Chemistry, Physical;Nanoscience & Nanotechnology;Materials Science, Multidisciplinary;Physics, Applied;Physics, Condensed Matter;Chemistry;Science & Technology - Other Topics;Materials Science;Physics;Perovskites;halides;quantum dots;rianoaystals;optoelectronies;LUMINESCENT SOLAR CONCENTRATORS;SHELL NANOCRYSTALS;S NANOCRYSTALS;CELLS;LIGHT;EFFICIENCY;EMERGENCE;DISPLAYS;Perovskites;halides;nanocrystals;optoelectronics;quantum dots;Nanoscience & Nanotechnology;MD Multidisciplinary
Issue Date: 22-Feb-2017
29-Jan-2015
1-Jan-2015
Publisher: American Chemical Society
Description: Metal halides perovskites, such as hybrid organic???inorganic CH3NH3PbI3, are newcomer optoelectronic materials that have attracted enormous attention as solution-deposited absorbing layers in solar cells with power conversion efficiencies reaching 20%. Herein we demonstrate a new avenue for halide perovskites by designing highly luminescent perovskite-based colloidal quantum dot materials. We have synthesized monodisperse colloidal nanocubes (4???15 nm edge lengths) of fully inorganic cesium lead halide perovskites (CsPbX3, X = Cl, Br, and I or mixed halide systems Cl/Br and Br/I) using inexpensive commercial precursors. Through compositional modulations and quantum size-effects, the bandgap energies and emission spectra are readily tunable over the entire visible spectral region of 410???700 nm. The photoluminescence of CsPbX3 nanocrystals is characterized by narrow emission line-widths of 12???42 nm, wide color gamut covering up to 140% of the NTSC color standard, high quantum yields of up to 90%, and radiative lifetimes in the range of 1???29 ns. The compelling combination of enhanced optical properties and chemical robustness makes CsPbX3 nanocrystals appealing for optoelectronic applications, particularly for blue and green spectral regions (410???530 nm), where typical metal chalcogenide-based quantum dots suffer from photodegradation.
URI: http://dx.doi.org/10.1021/nl5048779
Other Identifiers: http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcApp=PARTNER_APP&SrcAuth=LinksAMR&KeyUT=WOS:000356316900006&DestLinkType=FullRecord&DestApp=ALL_WOS&UsrCustomerID=1ba7043ffcc86c417c072aa74d649202
1530-6992
http://hdl.handle.net/10044/1/44320
Type Of Material: Other
Appears in Collections:Faculty of Engineering

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